Neutron Flux Variation at the Inner Irradiation Channel of the Nigeria Research Reactor-1 (NIRR-1)

Authors

  • Y. Musa Nuclear Science and Technology Section, Centre for Energy Research and Training, Ahmadu Bello University, Zaria, Nigeria
  • Y.A. Ahmed Nuclear Science and Technology Section, Centre for Energy Research and Training, Ahmadu Bello University, Zaria, Nigeria
  • Y.A. Yamusa Nuclear Science and Technology Section, Centre for Energy Research and Training, Ahmadu Bello University, Zaria, Nigeria
  • M. Tukur Nuclear Science and Technology Section, Centre for Energy Research and Training, Ahmadu Bello University, Zaria, Nigeria

DOI:

https://doi.org/10.6000/1929-6002.2014.03.04.3

Keywords:

Nuclear Flux, Irradiation Channel, NAA. NIRR-1.

Abstract

In order to ascertain the level of flux variation in one of the inner irradiation channels of the Nigeria Research Reactor-1 (NIRR-1), the irradiation container used for routine activation analysis was employed with copper wires as flux monitors. Measurements were carried out with these wires arranged in axial direction to determine the thermal neutron flux at selected positions using absolute foil activation method. Our results show that there exists a slight flux variation from one position to another ranging from (4.57 ± 0.24) x 1011 to (5.20 ± 0.20) x 1011 cm-2s-1. Individual foil shows slight flux variation from one position to another in the same irradiation container but they all pointed toward a level of stability in spite of the recent installation of the cadmium lined irradiation channel. The values obtained in this work are in good agreement with the previously measured value of (5.14 ± 0.24) x 1011 cm-2s-1 after commissioning of NIRR-1. This shows that the cadmium lined installation does not affect the flux stability. In order to improve the accuracy of neutron activation analysis (NAA) using NIRR-1 facility, there is need for flux corrections to be made by miniature neutron source reactor (MNSR) users during NAA particularly long irradiation, where more than six samples are irradiated simultaneously in the same container.

References

Jonah SA, Umar IM, Oladipo MOA, Balogun GI, Adeyemu DJ. Standardization of NIRR-1 irradiation and counting facilities for instrumental neutron activation analysis. Appl Rad Isot 2006; 64: 818-22. http://dx.doi.org/10.1016/j.apradiso.2006.01.012

Kapsimalis R, Landsberger S, Ahmed YA. The determination of uranium in food samples by Compton suppression epithermal neutron activation analysis. Appl Rad Isot 2009; 67: 2097-9. http://dx.doi.org/10.1016/j.apradiso.2009.05.011

Ahmed YA, Landsberger S, O’Kelly DJ, Braisted J, Gabdo H, Ewa IOB. Compton suppression method and epithermal NAA in the determination of nutrients and heavy metals in Nigeria food and beverages. Appl Rad Isot 2010; 68: 1909-14. http://dx.doi.org/10.1016/j.apradiso.2010.04.016

Acharya RN, Nair AGC, Reddy AVR, Manohar SB. Validation of a neutron activation analysis method using k0-standardization. Appl Rad Isot 2002; 57: 391-8. http://dx.doi.org/10.1016/S0969-8043(02)00111-2

Bode P, Blaauw M, Obrusnik I. Variation of neutron flux and related parameters in an irradiation container, in use with k0-based neutron activation analysis. J Radioanal Nucl Chem 1992; 157: 301-12. http://dx.doi.org/10.1007/BF02047445

Ahmed YA, Ewa IOB, Umar IM. Effective resonance energy and non-ideality of epithermal neutron flux distribution in neutron activation analysis. Nig J Phys 2002; 14: 82-5.

Parry SJ. Activation spectrometry in chemical analysis. John Wiley & Sons. 1991; New York.

Guosheng Z. Absolute neutron flux measurement by gold foil activation method, MNSR Training Material. 1993; China Institute of Atomic Energy.

Kafala SI, MacMahon TD. Comparison of neutron activation analysis methods. J Radioanal Nucl Chem 2007; 271: 507-16. http://dx.doi.org/10.1007/s10967-007-0238-6

Ahmed YA, Ewa IOB, Umar IM. Variations in nuclear data and its impact on INAA. J Appl Sci 2006; 6: 1692-7. http://dx.doi.org/10.3923/jas.2006.1692.1697

Abrefah RG, Nyarko BJB, Akaho EHK, Anim Sampong S, Sogbadji RBM. Axial and radial distribution of thermal and epithermal neutron fluxes in irradiation channels of the Ghana Research Reactor-1 using foil activation analysis. Ann Nucl Energy 2010; 37: 1027-35. http://dx.doi.org/10.1016/j.anucene.2010.04.017

Jonah SA, Balogun GI, Umar IM, Mayaki MC. Neutron spectrum parameters in irradiation channel of the Nigeria Research Reactor-1 (NIRR-1) for the k0-NAA standardization. J Radioanal Nucl Chem 2005; 226: 83-8. http://dx.doi.org/10.1007/s10967-005-0873-8

El-Khayatt AM. Elemental analysis of Egyptian crude oils by INAA using rabbit irradiation system at ETRR-2 reactor. Appl Rad Isot 2010; 68: 2438-42. http://dx.doi.org/10.1016/j.apradiso.2010.07.013

Moen L, De Corte F, Simonits A, Wispelaere A, Hoste J. The effective resonance energy Er as a parameter for the correction of resonance integrals, 1/E(1+α)epithermal neutron spectra: tabulation of Er for 96 isotopes. J Analyt Chem 1979; 52: 379-87.

Mustafa K, Haluk Y, Mustafa T, Atilla O. Measurement of thermal neutron cross-sections and resonance integrals for 71Ga(n,)72Ga and 75As(n,) 76As by using 241Am-Be isotopic neutron source. Nucl Instr Meth Phys Resear A 2003; 501: 524-35. http://dx.doi.org/10.1016/S0168-9002(03)00408-X

Menno B. The k0-Consistent IRI Gamma-ray Catalogue for Instrumental Neutron Activation Analysis. 1996; ISBN 90-73861-32-2: Interfaculty Reactor Institute Delft.

IAEA. Practical Aspects of Operating a Neutron Activation Analysis Laboratory, IAEA-TECDOC-564. 1990; ISSN 1011-4289: IAEA, Vienna.

Jonah SA, Ibrahim YV, Akaho EHK. The determination of reactor spectrum-averaged cross-sections in miniature neutron source reactor facility. Appl Rad Isot 2008; 66: 1377-80. http://dx.doi.org/10.1016/j.apradiso.2008.04.001

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Published

2014-12-08

How to Cite

Musa, Y., Ahmed, Y., Yamusa, Y., & Tukur, M. (2014). Neutron Flux Variation at the Inner Irradiation Channel of the Nigeria Research Reactor-1 (NIRR-1). Journal of Technology Innovations in Renewable Energy, 3(4), 171–176. https://doi.org/10.6000/1929-6002.2014.03.04.3

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